The error message is indicating that you have a client system (10.35.19.21) that is attempting to access a share in one of your EVS using SMB2 (the protocol, not necessarily the dialect, could be smb2, smb3, etc) but it is not providing valid signing against the current Domain.
Most likely it is providing credentials that do not valid in the current/new Active Directory. The message also indicates that it is attempting this access once every 10 seconds (120 min / 666 attempts). Best bet would be to review your client at 10.35.19.21 for automated/scheduled tasks or applications that attempt to access UNC paths and double check the credentials being used.